Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents

Natural-based hydrogels are popular due to their biodegradation ability compared to synthetic-based hydrogels which are more environmentally sustainable. However, natural-based hydrogels exhibit slow degradation and may require an enhancer to accelerate the degradation process. In this study, deep e...

وصف كامل

التفاصيل البيبلوغرافية
الحاوية / القاعدة:Journal of Advanced Research in Fluid Mechanics and Thermal Sciences
المؤلف الرئيسي: 2-s2.0-86000069247
التنسيق: مقال
اللغة:English
منشور في: Semarak Ilmu Publishing 2025
الوصول للمادة أونلاين:https://www.scopus.com/inward/record.uri?eid=2-s2.0-86000069247&doi=10.37934%2farfmts.127.2.6276&partnerID=40&md5=b99c81da7fb1b164c274ce70e706c211
id Md Raffe S.N.A.; Mohamed Hanaphi R.; Yusof R.
spelling Md Raffe S.N.A.; Mohamed Hanaphi R.; Yusof R.
2-s2.0-86000069247
Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
2025
Journal of Advanced Research in Fluid Mechanics and Thermal Sciences
127
2
10.37934/arfmts.127.2.6276
https://www.scopus.com/inward/record.uri?eid=2-s2.0-86000069247&doi=10.37934%2farfmts.127.2.6276&partnerID=40&md5=b99c81da7fb1b164c274ce70e706c211
Natural-based hydrogels are popular due to their biodegradation ability compared to synthetic-based hydrogels which are more environmentally sustainable. However, natural-based hydrogels exhibit slow degradation and may require an enhancer to accelerate the degradation process. In this study, deep eutectic solvent (DES) has been added as an enhancer to increase the process of biodegradation in pectin-chitosan hydrogels. The study has investigated the biodegradability of this new hydrogel after being modified with three different hydrogen bond donors (HBD) in DESs by measuring weight loss through the soil burial method. The results show the pectin and chitosan hydrogel with the addition of DESs known as eutectogels have a higher percentage of weight loss compared to their control (without DES). Eutectogels with different HBDs which are ethylene glycol, glycerol, and acetic acid are recorded as 76.02%, 72.14%, and 86.21% weight loss, respectively, while their control recorded 65.11% of weight loss in soil burial testing for 148 days. The addition of DES in pectin-chitosan-based hydrogel accelerates the degradation and improves the biodegradability of the eutectogel in soil. This demonstrates the potential of these eutectogels as biodegradable materials, offering promising applications in environmentally sensitive fields. © 2025, Semarak Ilmu Publishing. All rights reserved.
Semarak Ilmu Publishing
22897879
English
Article

author 2-s2.0-86000069247
spellingShingle 2-s2.0-86000069247
Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
author_facet 2-s2.0-86000069247
author_sort 2-s2.0-86000069247
title Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
title_short Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
title_full Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
title_fullStr Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
title_full_unstemmed Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
title_sort Enhanced Biodegradability of Pectin-Chitosan Eutectogels Synthesized with Deep Eutectic Solvents
publishDate 2025
container_title Journal of Advanced Research in Fluid Mechanics and Thermal Sciences
container_volume 127
container_issue 2
doi_str_mv 10.37934/arfmts.127.2.6276
url https://www.scopus.com/inward/record.uri?eid=2-s2.0-86000069247&doi=10.37934%2farfmts.127.2.6276&partnerID=40&md5=b99c81da7fb1b164c274ce70e706c211
description Natural-based hydrogels are popular due to their biodegradation ability compared to synthetic-based hydrogels which are more environmentally sustainable. However, natural-based hydrogels exhibit slow degradation and may require an enhancer to accelerate the degradation process. In this study, deep eutectic solvent (DES) has been added as an enhancer to increase the process of biodegradation in pectin-chitosan hydrogels. The study has investigated the biodegradability of this new hydrogel after being modified with three different hydrogen bond donors (HBD) in DESs by measuring weight loss through the soil burial method. The results show the pectin and chitosan hydrogel with the addition of DESs known as eutectogels have a higher percentage of weight loss compared to their control (without DES). Eutectogels with different HBDs which are ethylene glycol, glycerol, and acetic acid are recorded as 76.02%, 72.14%, and 86.21% weight loss, respectively, while their control recorded 65.11% of weight loss in soil burial testing for 148 days. The addition of DES in pectin-chitosan-based hydrogel accelerates the degradation and improves the biodegradability of the eutectogel in soil. This demonstrates the potential of these eutectogels as biodegradable materials, offering promising applications in environmentally sensitive fields. © 2025, Semarak Ilmu Publishing. All rights reserved.
publisher Semarak Ilmu Publishing
issn 22897879
language English
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